Unique Adsorption Properties of Cationic Dyes Malachite Green and Rhodamine-B on Longan (Dimocarpus longan) Peel
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Keywords:
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Bioadsorbent, Longan, Malachite Green, Rhodamine-B, Adsorption
Abstract
This research converts agricultural waste Longan (Dimocarpus longan) Peel is used in the adsorption process to reduce cationic dyes rhodamine-B and malachite green contaminants from aqueous solution. Longan (Dimocarpus longan) Peel was characterized by FT-IR, analysis XRD, SEM, BET, and TG-DTA. The characterization results show that Longan (Dimocarpus longan) Peel contains cellulose compounds and has a specific surface area 17.175 m2/g, with this Longan (Dimocarpus longan) Peel has the potential as a bio adsorbent. The adsorption capacity is proven by adsorption capacity (Qm) shows that the bioadsorbent adsorption of malachite green has a large adsorption capacity of 182.64 mg/g, while the adsorption capacity of rhodamine-B (Qm) reaches 52.557 mg/g and this bioadsorbent longan (Dimocarpus longan) peel is effective the adsorption was stable until the third cycle.
References
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Kurniawaty, D. (2019). Effect of Cadmium in Biosorption of Lead by Lengkeng Seed and Shell (Euphoria logan lour). Journal of Chemical Natural Resources, 1(2); 23–29
Kusrini, E., Kinastiti, D. D., Wilson, L.D., Usman, A., Rahman, A (2019). Adsorption of Lanthanide Ions from an Aque- ous Solution in Multicomponent Systems using Activated Carbon from Banana Peels (Musa Paradisiaca L.). Journal of Chemical Natural Resources, 19; 1132–1139
Lesbani, A., N. R. Palapa, R. J. Sayeri, T. Taher, and N. Hiday- ati (2021). High Reusability of NiAl LDH/Biochar Compos- ite in the Removal Methylene Blue from Aqueous Solution. Indonesian Journal of Chemistry, 21(2); 421-434
Lestari, N. A. (2019). Reduction of CO2 Emission by Inte- grated Biomass Gasification-Solid Oxide Fuel Cell Com- bined with Heat Recovery and in-situ CO2 Utilization. Ev- ergreen, 6(3); 254–261
Ma, J., L. Hou, P. Li, S. Zhang, and X. Zheng (2021). Modified Fruit Pericarp as an Effective Biosorbent for Removing Azo Dye from Aqueous Solution: Study of Adsorption Properties and Mechanisms. Environmental Engineering Research, 27(2); 200634
Mamat, M., M. A. A. Abdullah, M. A. Kadir, A. M. Jaafar, and E. Kusrini (2018). Preparation of Layered Double Hy- droxides with Different Divalent Metals for The Adsorption of Methyl Orange Dye from Aqueous Solutions. Chemical Engineering, 9(6); 1103–1111
Mishra, S., S. Sahoo, A. Debnath, K. Muthe, N. Das, and P. Parhi (2020). Cobalt Ferrite Nanoparticles Prepared by Microwave Hydrothermal Synthesis and Adsorption Effi- ciency for Organic Dyes: Isotherms, Thermodynamics and Kinetic Studies. Advanced Powder Technology, 31(11); 4552– 4562
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Onder, A., P. Ilgin, H. Ozay, and O. Ozay (2020). Removal of Dye from Aqueous Medium with pH-Sensitive Poly [(2- (acryloyloxy) ethyl] Trimethylammonium Chloride-co-1- vinyl-2-pyrrolidone] Cationic Hydrogel. Journal of Environ- mental Chemical Engineering, 8(5); 104436
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Priyanto, A., F, M., Muhdarina, M., A, A.(2021). Adsorption and Characterization of Activated Sugarcane Bagasse Using Natrium Hydroxide Indonesian Journal Chemical Research, 8; 202-209
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Rahmanian, O., M. Dinari, and M. K. Abdolmaleki (2018). Carbon Quantum Dots/Layered Double Hydroxide Hybrid for Fast and Efficient Decontamination of Cd (II): The Ad- sorption Kinetics and Isotherms. Applied Surface Science, 428; 272–279
Satya, A., Harimawan, A., Haryani, G. S., Johir, M. A. H., Vi- gneswaran, S., Ngo, H. H., Setiadi, T (2020). Batch Study of
Cadmium Biosorption by Carbon Dioxide Enriched Aphan- othece sp. Dried Biomass. Water, 12; 1–10
Shaikhiev, I. G., N. V. Kraysman, and S. V. Sverguzova (2022). Onion (Allium Cepa) Processing Waste as a Sorption Material for Removing Pollutants from Aqueous Media. Biointerface Research in Applied Chemistry, 12(3); 3173–3185
Tariq, M., M. Muhammad, J. Khan, A. Raziq, M. K. Uddin, A. Niaz, S. S. Ahmed, and A. Rahim (2020). Removal of Rhodamine B dye from Aqueous Solutions using Photo- Fenton Processes and Novel Ni-Cu@ MWCNTs Photocata- lyst. Journal of Molecular Liquids, 312; 113399
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Tongpoothorn, W., O. Somsimee, T. Somboon, and M. Sriut- tha (2019). An Alternative and Cost-Effective Biosorbent Derived from Napier Grass Stem for Malachite Green Re- moval. Journal of Materials and Environmental Sciences, 10(8); 685–695
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Wang, L., A. Li, and Y. Chang (2016a). Hydrothermal Treat- ment Coupled with Mechanical Expression at Increased Temperature for Excess Sludge Dewatering: Heavy Met- als, Volatile Organic Compounds and Combustion Charac- teristics of Hydrochar. Chemical Engineering Journal, 297; 1–10
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Wijaya, A., P. M. S. B. N. Siregar, A. Priambodo, N. R. Palapa, T. Taher, and A. Lesbani (2021). Innovative Modified of Cu-Al/C (C= Biochar, Graphite) Composites for Removal of Procion Red from Aqueous Solution. Science and Technology Indonesia, 6(4); 228–234
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Ahmed, D. N., L. A. Naji, A. A. Faisal, N. Al-Ansari, and M. Naushad (2020). Waste Foundry Sand/MgFe-Layered Double Hydroxides Composite Material for Efficient Re- moval of Congo Red Dye from Aqueous Solution. Scientific Reports, 10(1); 1–12
Alam, M. A. and K. Al Riyami (2018). Shear Strengthening of Reinforced Concrete Beam using Natural Fibre Reinforced Polymer Laminates. Construction and Building Materials, 162; 683–696
Albo, J., M. I. Qadir, M. Samperi, J. A. Fernandes, I. de Pedro, and J. Dupont (2021). Use of an Optofluidic Microreactor and Cu Nanoparticles Synthesized in Ionic Liquid and Em- bedded in TiO2 for an Efficient Photoreduction of CO2 to Methanol. Chemical Engineering Journal, 404; 126643
Ali, F., N. Ali, I. Bibi, A. Said, S. Nawaz, Z. Ali, S. M. Salman, H. M. Iqbal, and M. Bilal (2020). Adsorption Isotherm, Kinetics and Thermodynamic of Acid Blue and Basic Blue Dyes onto Activated Charcoal. Case Studies in Chemical and Environmental Engineering, 2(9); 100040
Biesinger, M. C., B. P. Payne, A. P. Grosvenor, L. W. Lau, A. R. Gerson, and R. S. C. Smart (2011). Resolving Surface Chemical States in XPS Analysis of First Row Transition Metals, Oxides and Hydroxides: Cr, Mn, Fe, Co and Ni. Applied Surface Science, 257(7); 2717–2730
Brame, J. A. and C. S. Griggs (2016). Surface Area Analysis using The Brunauer-Emmett-Teller (BET) Method: Scien- tific Operation Procedure Series: SOP-C. U.S Army Engineer Research and Development Center, 1; 1–23.
Chang, C. C. and R. Li (2019). Agricultural Waste. Water Environment Research, 91(10); 1150–1167
Chen, X., Q. Lin, R. He, X. Zhao, and G. Li (2017). Hydrochar Production from Watermelon Peel by Hydrothermal Car- bonization. Bioresource Technology, 241; 236–243
Cheng, Z.L., Y. X. Li, and Z. Liu (2018). Study on Adsorption of Rhodamine B onto Beta Zeolites by Tuning SiO2/Al2O3 ratio. Ecotoxicology and Environmental Safety, 148; 585–592
Dang, W., J. Zhang, H. Nie, F. Wang, X. Tang, N. Wu, Q. Chen, X. Wei, and R. Wang (2020). Isotherms, Ther- modynamics and Kinetics of Methane-Shale Adsorption Pair Under Supercritical Condition: Implications for Un- derstanding The Nature of Shale Gas Adsorption Process. Chemical Engineering Journal, 383; 123191
Fan, X., Deng, L., Li, K., Lu, H., Wang, R., and Li, W (2021). Adsorption of Malachite Green in Aqueous Solution using Sugarcane Bagasse-Barium Carbonate Composite Colloids and Interface Science Communications, 44; 100485
Grabi, H., F. Derridj, W. Lemlikchi, and E. Guénin (2021). Studies of The Potential of a Native Natural Biosorbent for The Elimination of An Anionic Textile Dye Cibacron Blue in Aqueous Solution. Scientific Reports, 11(1); 1–13
Ikhtiari, R., H. Aziz, R. Zein, et al. (2015). The Removal of Cr(VI) with Dimocarpus longan as a Low Cost Biosorbent. Journal of Chemical and Pharmaceutical Research, 7(9S); 81–88
Ismail, S. N. A. S., W. A. Rahman, N. A. A. Rahim, N. D. Masdar, and M. L. Kamal (2018). Adsorption of Malachite Green dye From Aqueous Solution using Corncob. In AIP Conference Proceedings, 2031; 020036
Juleanti, N., N. R. Palapa, T. Taher, N. Hidayati, B. I. Putri, and A. Lesbani (2021). The Capability of Biochar-Based CaAl and MgAl Composite Materials as Adsorbent for Re- moval Cr (VI) in Aqueous Solution. Science and Technology Indonesia, 6(3); 196–203
Kalak, T., J. Walczak, and M. Ulewicz (2021). Adsorptive Recovery of Cd (II) Ions with The Use of Post-Production Waste Generated in the Brewing Industry. Energies, 14(17); 5543
Karthikeyan, P. and S. Meenakshi (2020). Enhanced Removal of Phosphate and Nitrate Ions by a Novel ZnFe LDHs- Activated Carbon Composite. Sustainable Materials and Tech- nologies, 25; e00154
Kaykhaii, M., M. Sasani, and S. Marghzari (2018). Removal of Dyes from The Environment by Adsorption Process. Chem- ical and Materials Engineering, 6(2); 31–35
Krishni, R., K. Foo, and B. Hameed (2014). Food Cannery
Effluent, Pineapple Peel as an Efective Low-Cost Biosor- bent for Removing Cationic Dye from Aqueous Solutions. Desalination and Water Treatment, 52(31-33); 6096–6103
Kumari, S., A. A. Khan, A. Chowdhury, A. K. Bhakta, Z. Mekhalif, and S. Hussain (2020). Efficient and Highly Selective Adsorption of Cationic Dyes and Removal of Ciprofloxacin Antibiotic by Surface Modified Nickel Sulfide Nanomaterials: Kinetics, Isotherm and Adsorption Mecha- nism. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 586; 124264
Kurniawati, D., T. Sari, F. Adella, S. Sy, et al. (2021). Effect of Contact Time Adsorption of Rhodamine B, Methyl Or- ange and Methylene Blue Colours on Langsat Shell with Batch Methods. In Journal of Physics: Conference Series, 1788; 012008
Kurniawaty, D. (2019). Effect of Cadmium in Biosorption of Lead by Lengkeng Seed and Shell (Euphoria logan lour). Journal of Chemical Natural Resources, 1(2); 23–29
Kusrini, E., Kinastiti, D. D., Wilson, L.D., Usman, A., Rahman, A (2019). Adsorption of Lanthanide Ions from an Aque- ous Solution in Multicomponent Systems using Activated Carbon from Banana Peels (Musa Paradisiaca L.). Journal of Chemical Natural Resources, 19; 1132–1139
Lesbani, A., N. R. Palapa, R. J. Sayeri, T. Taher, and N. Hiday- ati (2021). High Reusability of NiAl LDH/Biochar Compos- ite in the Removal Methylene Blue from Aqueous Solution. Indonesian Journal of Chemistry, 21(2); 421-434
Lestari, N. A. (2019). Reduction of CO2 Emission by Inte- grated Biomass Gasification-Solid Oxide Fuel Cell Com- bined with Heat Recovery and in-situ CO2 Utilization. Ev- ergreen, 6(3); 254–261
Ma, J., L. Hou, P. Li, S. Zhang, and X. Zheng (2021). Modified Fruit Pericarp as an Effective Biosorbent for Removing Azo Dye from Aqueous Solution: Study of Adsorption Properties and Mechanisms. Environmental Engineering Research, 27(2); 200634
Mamat, M., M. A. A. Abdullah, M. A. Kadir, A. M. Jaafar, and E. Kusrini (2018). Preparation of Layered Double Hy- droxides with Different Divalent Metals for The Adsorption of Methyl Orange Dye from Aqueous Solutions. Chemical Engineering, 9(6); 1103–1111
Mishra, S., S. Sahoo, A. Debnath, K. Muthe, N. Das, and P. Parhi (2020). Cobalt Ferrite Nanoparticles Prepared by Microwave Hydrothermal Synthesis and Adsorption Effi- ciency for Organic Dyes: Isotherms, Thermodynamics and Kinetic Studies. Advanced Powder Technology, 31(11); 4552– 4562
Moghadam, M. R., N. Nasirizadeh, Z. Dashti, and E. Ba- banezhad (2013). Removal of Fe(II) from Aqueous Solution using Pomegranate Peel Carbon: Equilibrium and Kinetic Studies. International Journal of Industrial Chemistry, 4(1); 1–6
Moller, M., and Pich, A (2017). Development of Modified Layered Silicates with Superior Adsorption Properties for Uptake of Pollutants from Air and Water. Development of Modified Layered Silicates with Superior Adsorption Prop- erties for Uptake of Pollutants from Air and Water Von. Disertation; University Zur Erlangung Des
Moosa, A., Ridha, A., Moosa, A.A., Ridha, A.M., Hussien, N.A (2016). Removal of Zinc Ions from Aqueous Solution by Bioadsorbents and CNTs Removal of Zinc Ions from Aqueous Solution by Bioadsorbents and CNTs. International Journal of Industrial Chemistry, 5; 1–10
Neolaka, Y. A., Y. Lawa, J. N. Naat, A. A. Riwu, M. Iqbal, H. Darmokoesoemo, and H. S. Kusuma (2020). The Ad- sorption of Cr(VI) from Water Samples using Graphene Oxide-Magnetic (GO-Fe3O4) Synthesized from Natural Cellulose-Based Graphite (Kusambi Wood or Schleichera oleosa): Study of Kinetics, Isotherms and Thermodynam- ics. Journal of Materials Research and Technology, 9(3); 6544– 6556
Nor, N. M., T. Hadibarata, Z. Yusop, and Z. M. Lazim (2015). Removal of Brilliant Green and Procionred Dyes from Aqueous Solution by Adsorption using Selected Agricultural Wastes. Jurnal Teknologi, 74(11); 117–122
Normah, N., N. Juleanti, P. M. S. B. N. Siregar, A. Wijaya, N. R. Palapa, T. Taher, and A. Lesbani (2021). Size Selec- tivity of Anionic and Cationic Dyes Using LDH Modified Adsorbent with Low-Cost Rambutan Peel to Hydrochar. Bulletin of Chemical Reaction Engineering & Catalysis, 16(4); 869–880
Oliveira, E., J. Santos, A. Goncalves, S. Mattedi, and N. Jose (2016). Characterization of The Rambutan Peel Fiber (Nephelium lappaceum) as a Lignocellulosic Material for Tech- nological Applications. Chemical Engineering Transactions, 50; 391–396
Onder, A., P. Ilgin, H. Ozay, and O. Ozay (2020). Removal of Dye from Aqueous Medium with pH-Sensitive Poly [(2- (acryloyloxy) ethyl] Trimethylammonium Chloride-co-1- vinyl-2-pyrrolidone] Cationic Hydrogel. Journal of Environ- mental Chemical Engineering, 8(5); 104436
Pathak, P.D., Mandavgane, S.A., Kulkarni, B.D. (2015). Fruit Peel Waste as a Novel Low-Cost Biodsorbent. Reviews in Chemical Engineering, 31; 361-381
Priyanto, A., F, M., Muhdarina, M., A, A.(2021). Adsorption and Characterization of Activated Sugarcane Bagasse Using Natrium Hydroxide Indonesian Journal Chemical Research, 8; 202-209
Qu, W., T. Yuan, G. Yin, S. Xu, Q. Zhang, and H. Su (2019). Effect of Properties of Activated Carbon on Malachite Green Adsorption. Fuel, 249; 45–53
Rahmanian, O., M. Dinari, and M. K. Abdolmaleki (2018). Carbon Quantum Dots/Layered Double Hydroxide Hybrid for Fast and Efficient Decontamination of Cd (II): The Ad- sorption Kinetics and Isotherms. Applied Surface Science, 428; 272–279
Satya, A., Harimawan, A., Haryani, G. S., Johir, M. A. H., Vi- gneswaran, S., Ngo, H. H., Setiadi, T (2020). Batch Study of
Cadmium Biosorption by Carbon Dioxide Enriched Aphan- othece sp. Dried Biomass. Water, 12; 1–10
Shaikhiev, I. G., N. V. Kraysman, and S. V. Sverguzova (2022). Onion (Allium Cepa) Processing Waste as a Sorption Material for Removing Pollutants from Aqueous Media. Biointerface Research in Applied Chemistry, 12(3); 3173–3185
Tariq, M., M. Muhammad, J. Khan, A. Raziq, M. K. Uddin, A. Niaz, S. S. Ahmed, and A. Rahim (2020). Removal of Rhodamine B dye from Aqueous Solutions using Photo- Fenton Processes and Novel Ni-Cu@ MWCNTs Photocata- lyst. Journal of Molecular Liquids, 312; 113399
Ting, A. S. Y., C. K. W. Cheng, and K. A. A. Santiago (2021). Decolourization of Malachite Green Dye by Endolichenic Fungi from The Lichen Usnea sp. : A Novel Study on Their Dye Removal Potential. Journal of King Saud University Sci- ence, 33(7); 101579
Tongpoothorn, W., O. Somsimee, T. Somboon, and M. Sriut- tha (2019). An Alternative and Cost-Effective Biosorbent Derived from Napier Grass Stem for Malachite Green Re- moval. Journal of Materials and Environmental Sciences, 10(8); 685–695
Vasu, A. E. (2007). Biosorption of Rhodamine B and Malachite Green from Aqueous Aolutions by Tamarindus Indica Fruit Shells. Current World Environment, 2(2); 127
Wang, L., A. Li, and Y. Chang (2016a). Hydrothermal Treat- ment Coupled with Mechanical Expression at Increased Temperature for Excess Sludge Dewatering: Heavy Met- als, Volatile Organic Compounds and Combustion Charac- teristics of Hydrochar. Chemical Engineering Journal, 297; 1–10
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Authors
Mohadi, R., Normah, Salasia Fitri, E., & Rahayu Palapa, N. (2022). Unique Adsorption Properties of Cationic Dyes Malachite Green and Rhodamine-B on Longan (Dimocarpus longan) Peel. Science and Technology Indonesia, 7(1), 115–125. https://doi.org/10.26554/sti.2022.7.1.115-125
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