Facile Fabrication of Layered Double Hydroxide-Lignin for Efficient Adsorption of Malachite Green
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Keywords:
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Layered Double Hydroxide, Adsorption, Lignin, Malachite Green
Abstract
Preparation of layered double hydroxide-lignin (lignin-Zn/Al) carried out by coprecipitation method. The FTIR spectra of lignin-Zn/Al displayed at 3448, 2939, 1620, 1381, 1118, 1041, and 601 cm−1. The characteristic peaks are located at 10.1°, 19.1°, 20.1°, 29.4°, 33.9°, and 60.4°. The lignin-Zn/Al nitrogen adsorption-desorption isotherm showed a Type-IV curve, indicating that it had a mesoporous structure. The H3 kind of hysteresis loop also provides evidence for the presence of mesopores within the lignin-Zn/Al complex. Lignin-Zn/Al, lignin, and Zn/Al had pHpzc values of 6.09, 3.01, and 6.09, respectively. Lignin-Zn/Al, lignin, and Zn/Al are positively charged when the pH of the solution is less than pHpzc, and they are negatively charged when the pH of the solution is more than pHpzc. The Langmuir and pseudo-second-order model best represented the MG adsorption onto all adsorbents. The lignin-Zn/Al, lignin, and Zn/Al were shown to have maximum Langmuir adsorption capacities of 83.034, 78.740, and 36.364 mg/g, respectively. Zn/Al adsorption capacity increased 2.28 times after being composited with lignin.
References
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Heo, J. W., L. An, J. Chen, J. H. Bae, and Y. S. Kim (2022). Preparation of Amine-functionalized Lignins for the Selective Adsorption of Methylene Blue and Congo Red. Chemosphere, 295; 133815
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Jin, C., Y. Liu, J. Fan, T. Liu, G. Liu, F. Chu, and Z. Kong (2022). Lignin-inspired Porous Polymer Networks as High-performance Adsorbents for the Efficient Removal of Malachite Green Dye. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 643; 128760
Juleanti, N., N. R. Palapa, T. Taher, N. Hidayati, B. I. Putri, and A. Lesbani (2021). The Capability of Biochar-based CaAl and MgAl Composite Materials as Adsorbent For Removal Cr (VI) in Aqueous Solution. Science and Technology Indonesia, 6(3); 196–203
Kavci, E. (2021). Malachite Green Adsorption Onto Modified Pine Cone: Isotherms, Kinetics and Thermodynamics Mechanism. Chemical Engineering Communications, 208(3); 318–327
Meng, Z., M. Wu, S. Zhao, R. Jing, S. Li, Y. Shao, X. Liu, F. Lv, A. Liu, and Q. Zhang (2019). Removing Anionic Dyes from Wastewater Based on In-situ Formation Of Fe3O4@ Zn-Al Layered Double Hydroxides by Self-assembly. Applied Clay Science, 170; 41–45
Moradi, O. and S. Panahandeh (2022). Fabrication of Different Adsorbents Based on Zirconium Oxide, Graphene Oxide, and Dextrin for Removal of Green Malachite Dye from Aqueous Solutions. Environmental Research, 214; 114042
Muinde, V. M., J. M. Onyari, B. Wamalwa, and J. N. Wabomba (2020). Adsorption of Malachite Green Dye From Aqueous Solutions Using Mesoporous Chitosan–zinc Oxide Composite Material. Environmental Chemistry and Ecotoxicology, 2; 115–125
Nazir, M. A., T. Najam, S. Jabeen, M. A. Wattoo, M. S. Bashir, S. S. A. Shah, and A. ur Rehman (2022). Facile Synthesis of Tri-metallic Layered Double Hydroxides (NiZnAl-LDHs): Adsorption of Rhodamine-B and Methyl Orange from Water. Inorganic Chemistry Communications, 145; 110008
Pathania, D., V. S. Bhat, J. M. Shivanna, G. Sriram, M. Kurkuri, and G. Hegde (2022). Garlic Peel Based Mesoporous Carbon Nanospheres for an Effective Removal of Malachite Green Dye from Aqueous Solutions: Detailed Isotherms and Kinetics. Spectrochimica Acta Part A: Molecular and Biomolecular Spectroscopy, 276; 121197
Puthukkara, P., A. Rose, T. S. Jose, and S. D. Lal (2022). Green Synthesis of Iron Nanoparticles for Malachite Green Removal. Materials Today Communications, 33(4); 50–60
Rashed, S. H., A. Abd Elhamid, S. Y. H. Abdalkarim, R. H. El Sayed, A. A. El Bardan, H. M. Soliman, and A. Nayl (2022). Preparation and Characterization of Layered Double Hydroxides Decorated on Graphene Oxide For Dye Removal from Aqueous Solution. Journal of Materials Research and Technology, 17; 2782–2795
Raval, A. R., H. P. Kohli, and O. K. Mahadwad (2022). Application of Emulsion Liquid Membrane for Removal of Malachite Green Dye from Aqueous Solution: Extraction and Stability Studies. Chemical Engineering Journal Advances, 12; 100398
Ren, Q., C. Kong, Z. Chen, J. Zhou, W. Li, D. Li, Z. Cui, Y. Xue, and Y. Lu (2021). Ultrasonic Assisted Electrochemical Degradation of Malachite Green In Wastewater. Microchemical Journal, 164; 106059
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Sun, Y., T. Wang, C. Han, X. Lv, L. Bai, X. Sun, and P. Zhang (2022). Facile Synthesis of Fe modified Lignin-based Biochar for Ultra-fast Adsorption of Methylene Blue: Selective Adsorption and Mechanism Studies. Bioresource Technology, 344; 126186
Tang, R., W. Hong, C. Srinivasakannan, X. Liu, X. Wang, and X. Duan (2022). A Novel Mesoporous Fe-silica Aerogel Composite with Phenomenal Adsorption Capacity for Malachite Green. Separation and Purification Technology, 281; 119950
Van Tran, T., D. T. C. Nguyen, P. S. Kumar, A. T. M. Din, A. S. Qazaq, and D. V. N. Vo (2022). Green Synthesis of Mn3O4 Nanoparticles Using Costus Woodsonii Flowers Extract for Effective Removal of Malachite Green Dye. Environmental Research, 214; 113925
Vigneshwaran, S., P. Sirajudheen, P. Karthikeyan, and S. Meenakshi (2021). Fabrication of Sulfur doped Biochar Derived from Tapioca Peel Waste with Superior Adsorption Performance for the Removal of Malachite Green and Rhodamine B Dyes. Surfaces and Interfaces, 23; 100920
Wang, T., M. Jiang, X. Yu, N. Niu, and L. Chen (2022). Application of Lignin Adsorbent in Wastewater Treatment: A Review. Separation and Purification Technology, 302; 122116
Wang, T., C. Li, C. Wang, and H. Wang (2018). Biochar/MnAl-LDH Composites for Cu (II) Removal from Aqueous Solution. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 538; 443–450
Yuliasari, N., A. Wijaya, R. Mohadi, and A. Lesbani (2023). Enhanced Effectiveness on Phenol Removal by MgCr-LDH/Microcrystalline Cellulose Composite and Regeneration Study with Green Desorption Reagent. Science and Technology Indonesia, 8(1); 151–159
Zong, E., R. Fan, H. Hua, J. Yang, S. Jiang, J. Dai, X. Liu, and P. Song (2023). A Magnetically Recyclable Lignin-based Bio-adsorbent for Efficient Removal of Congo Red From Aqueous Solution. International Journal of Biological Macromolecules, 226; 443–453
Zubair, M., H. A. Aziz, I. Ihsanullah, M. A. Ahmad, and M. A. Al Harthi (2022). Engineered Biochar Supported Layered Double Hydroxide-cellulose Nanocrystals Composite-: Synthesis, Characterization and Azo Dye Removal Performance. Chemosphere, 307; 136054
Ahmad, N., F. S. Arsyad, I. Royani, P. M. S. B. N. Siregar, T. Taher, and A. Lesbani (2023b). High Regeneration of ZnAl/NiAl-Magnetite Humic Acid for Adsorption of Congo Red from Aqueous Solution. Inorganic Chemistry Communications, 150; 110517
Ahmed, M. A. and A. A. Mohamed (2022). A Systematic Review of Layered Double Hydroxide based Materials for Environmental Remediation of Heavy Metals and Dye Pollutants. Inorganic Chemistry Communications, 148; 110325
Altun, T. and H. Ecevit (2022). Adsorption of Malachite Green and Methyl Violet 2B by Halloysite Nanotube: Batch Adsorption Experiments and Box-behnken Experimental Design. Materials Chemistry and Physics, 291; 126612
Banerjee, S., G. C. Sharma, R. K. Gautam, M. Chattopadhyaya, S. N. Upadhyay, and Y. C. Sharma (2016). Removal of Malachite Green, A Hazardous Dye from Aqueous Solutions Using Avena Sativa (oat) Hull as A Potential Adsorbent. Journal of Molecular Liquids, 213; 162–172
Buvaneswari, K. and M. Singanan (2022). Removal of Malachite Green Dye In Synthetic Wastewater Using Zingiber Officinale Plant Leaves Biocarbon. Materials Today: Proceedings, 55; 274–279
Chen, H., T. Liu, Y. Meng, Y. Cheng, J. Lu, and H. Wang (2020). Novel Graphene Oxide/Aminated Lignin Aerogels for Enhanced Adsorption of Malachite Green in Wastewater. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 603; 125281
Chen, Y., S. Chen, Z. Deng, X. Xu, J. Qin, X. Guo, Z. Bai, X. Chen, and Z. Lu (2022). Fabrication of Polystyrene/Cuo@ Calcined Layered Double Hydroxide Microspheres with High Adsorption Capacity for Congo Red. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 652; 129827
Dahlan, I., O. H. Keat, H. A. Aziz, and Y. T. Hung (2023). Synthesis and Characterization of MOF 5 Incorporated Waste derived Siliceous Materials for the Removal of Malachite Green Dye From Aqueous Solution. Sustainable Chemistry and Pharmacy, 31; 100954
Du, B., W. Li, L. Chai, W. Li, X. Wang, X. Chen, J. Zhou, and R. C. Sun (2023). Preparation of Versatile Lignin-based Adsorbent for The Removal of Organic Dyes and Its Application in Wound Healing. Journal of Molecular Liquids, 377; 121566
Giri, B. S., R. K. Sonwani, S. Varjani, D. Chaurasia, T. Varadavenkatesan, P. Chaturvedi, S. Yadav, V. Katiyar, R. S. Singh, and A. Pandey (2022). Highly Efficient Bio-adsorption of Malachite Green Using Chinese Fan-palm Biochar (livistona Chinensis). Chemosphere, 287; 132282
Hamad, H. A., S. AbdElhafez, M. Elsenety, M. K. Sorour, N. Amin, O. Abdelwahab, and E. Z. El Ashtoukhy (2022). Fabrication and Characterization of Functionalized Lignin-based Adsorbent Prepared from Black Liquor in the Paper Industry for Superior Removal of Toxic Dye. Fuel, 323; 124288
Hasan, I., D. Bhatia, S. Walia, and P. Singh (2020). Removal of Malachite Green by Polyacrylamide-g-chitosan ????-Fe2O3 Nanocomposite-an Application of Central Composite Design. Groundwater for Sustainable Development, 11; 100378
Heo, J. W., L. An, J. Chen, J. H. Bae, and Y. S. Kim (2022). Preparation of Amine-functionalized Lignins for the Selective Adsorption of Methylene Blue and Congo Red. Chemosphere, 295; 133815
Hijab, M., P. Parthasarathy, H. R. Mackey, T. Al Ansari, and G. McKay (2021). Minimizing Adsorbent Requirements Using Multi-stage Batch Adsorption for Malachite Green Removal Using Microwave Date-stone Activated Carbons. Chemical Engineering and Processing Process Intensification, 167; 108318
Iqbal, A., E. Cevik, A. Bozkurt, S. M. M. Asiri, O. Alagha, T. F. Qahtan, M. I. Jalees, and M. U. Farooq (2022). Ultrahigh Adsorption by Regenerable Iron-cobalt Core-shell Nanospheres and Their Synergetic Effect on Nanohybrid Membranes for Removal Of Malachite Green Dye. Journal of Environmental Chemical Engineering, 10(3); 107968
Jin, C., Y. Liu, J. Fan, T. Liu, G. Liu, F. Chu, and Z. Kong (2022). Lignin-inspired Porous Polymer Networks as High-performance Adsorbents for the Efficient Removal of Malachite Green Dye. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 643; 128760
Juleanti, N., N. R. Palapa, T. Taher, N. Hidayati, B. I. Putri, and A. Lesbani (2021). The Capability of Biochar-based CaAl and MgAl Composite Materials as Adsorbent For Removal Cr (VI) in Aqueous Solution. Science and Technology Indonesia, 6(3); 196–203
Kavci, E. (2021). Malachite Green Adsorption Onto Modified Pine Cone: Isotherms, Kinetics and Thermodynamics Mechanism. Chemical Engineering Communications, 208(3); 318–327
Meng, Z., M. Wu, S. Zhao, R. Jing, S. Li, Y. Shao, X. Liu, F. Lv, A. Liu, and Q. Zhang (2019). Removing Anionic Dyes from Wastewater Based on In-situ Formation Of Fe3O4@ Zn-Al Layered Double Hydroxides by Self-assembly. Applied Clay Science, 170; 41–45
Moradi, O. and S. Panahandeh (2022). Fabrication of Different Adsorbents Based on Zirconium Oxide, Graphene Oxide, and Dextrin for Removal of Green Malachite Dye from Aqueous Solutions. Environmental Research, 214; 114042
Muinde, V. M., J. M. Onyari, B. Wamalwa, and J. N. Wabomba (2020). Adsorption of Malachite Green Dye From Aqueous Solutions Using Mesoporous Chitosan–zinc Oxide Composite Material. Environmental Chemistry and Ecotoxicology, 2; 115–125
Nazir, M. A., T. Najam, S. Jabeen, M. A. Wattoo, M. S. Bashir, S. S. A. Shah, and A. ur Rehman (2022). Facile Synthesis of Tri-metallic Layered Double Hydroxides (NiZnAl-LDHs): Adsorption of Rhodamine-B and Methyl Orange from Water. Inorganic Chemistry Communications, 145; 110008
Pathania, D., V. S. Bhat, J. M. Shivanna, G. Sriram, M. Kurkuri, and G. Hegde (2022). Garlic Peel Based Mesoporous Carbon Nanospheres for an Effective Removal of Malachite Green Dye from Aqueous Solutions: Detailed Isotherms and Kinetics. Spectrochimica Acta Part A: Molecular and Biomolecular Spectroscopy, 276; 121197
Puthukkara, P., A. Rose, T. S. Jose, and S. D. Lal (2022). Green Synthesis of Iron Nanoparticles for Malachite Green Removal. Materials Today Communications, 33(4); 50–60
Rashed, S. H., A. Abd Elhamid, S. Y. H. Abdalkarim, R. H. El Sayed, A. A. El Bardan, H. M. Soliman, and A. Nayl (2022). Preparation and Characterization of Layered Double Hydroxides Decorated on Graphene Oxide For Dye Removal from Aqueous Solution. Journal of Materials Research and Technology, 17; 2782–2795
Raval, A. R., H. P. Kohli, and O. K. Mahadwad (2022). Application of Emulsion Liquid Membrane for Removal of Malachite Green Dye from Aqueous Solution: Extraction and Stability Studies. Chemical Engineering Journal Advances, 12; 100398
Ren, Q., C. Kong, Z. Chen, J. Zhou, W. Li, D. Li, Z. Cui, Y. Xue, and Y. Lu (2021). Ultrasonic Assisted Electrochemical Degradation of Malachite Green In Wastewater. Microchemical Journal, 164; 106059
Sarkar, S., N. Tiwari, A. Basu, M. Behera, B. Das, S. Chakrabortty, K. Sanjay, M. Suar, T. K. Adhya, and S. Banerjee (2021). Sorptive Removal of Malachite Green From Aqueous Solution by Magnetite/coir Pith Supported Sodium Alginate Beads: Kinetics, Isotherms, Thermodynamics and Parametric Optimization. Environmental Technology & Innovation, 24; 101818
Sturgeon, M. R., M. H. O’Brien, P. N. Ciesielski, R. Katahira, J. S. Kruger, S. C. Chmely, J. Hamlin, K. Lawrence, G. B. Hunsinger, and T. D. Foust (2014). Lignin Depolymerisation by Nickel Supported Layered Double Hydroxide Catalysts. Green Chemistry, 16(2); 824–835
Sun, Y., T. Wang, C. Han, X. Lv, L. Bai, X. Sun, and P. Zhang (2022). Facile Synthesis of Fe modified Lignin-based Biochar for Ultra-fast Adsorption of Methylene Blue: Selective Adsorption and Mechanism Studies. Bioresource Technology, 344; 126186
Tang, R., W. Hong, C. Srinivasakannan, X. Liu, X. Wang, and X. Duan (2022). A Novel Mesoporous Fe-silica Aerogel Composite with Phenomenal Adsorption Capacity for Malachite Green. Separation and Purification Technology, 281; 119950
Van Tran, T., D. T. C. Nguyen, P. S. Kumar, A. T. M. Din, A. S. Qazaq, and D. V. N. Vo (2022). Green Synthesis of Mn3O4 Nanoparticles Using Costus Woodsonii Flowers Extract for Effective Removal of Malachite Green Dye. Environmental Research, 214; 113925
Vigneshwaran, S., P. Sirajudheen, P. Karthikeyan, and S. Meenakshi (2021). Fabrication of Sulfur doped Biochar Derived from Tapioca Peel Waste with Superior Adsorption Performance for the Removal of Malachite Green and Rhodamine B Dyes. Surfaces and Interfaces, 23; 100920
Wang, T., M. Jiang, X. Yu, N. Niu, and L. Chen (2022). Application of Lignin Adsorbent in Wastewater Treatment: A Review. Separation and Purification Technology, 302; 122116
Wang, T., C. Li, C. Wang, and H. Wang (2018). Biochar/MnAl-LDH Composites for Cu (II) Removal from Aqueous Solution. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 538; 443–450
Yuliasari, N., A. Wijaya, R. Mohadi, and A. Lesbani (2023). Enhanced Effectiveness on Phenol Removal by MgCr-LDH/Microcrystalline Cellulose Composite and Regeneration Study with Green Desorption Reagent. Science and Technology Indonesia, 8(1); 151–159
Zong, E., R. Fan, H. Hua, J. Yang, S. Jiang, J. Dai, X. Liu, and P. Song (2023). A Magnetically Recyclable Lignin-based Bio-adsorbent for Efficient Removal of Congo Red From Aqueous Solution. International Journal of Biological Macromolecules, 226; 443–453
Zubair, M., H. A. Aziz, I. Ihsanullah, M. A. Ahmad, and M. A. Al Harthi (2022). Engineered Biochar Supported Layered Double Hydroxide-cellulose Nanocrystals Composite-: Synthesis, Characterization and Azo Dye Removal Performance. Chemosphere, 307; 136054
Authors
Palapa, N. R., Ahmad, N., Wijaya, A., & Zahara, Z. A. (2023). Facile Fabrication of Layered Double Hydroxide-Lignin for Efficient Adsorption of Malachite Green. Science and Technology Indonesia, 8(2), 305–311. https://doi.org/10.26554/sti.2023.8.2.305-311
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