Improvement of Congo Red Photodegradation Performance Through Zn/Al-TiO2 and Zn/Al-ZnO Preparation
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Keywords:
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Zn/Al LDH, Congo Red, ZnO, TiO2, Photodegradation
Abstract
Layered double hydroxide (LDH) is an anionic clay material known to be effective as a catalyst for the photodegradation of dye organic pollutants. Zn/Al LDH was synthesized by coprecipitation then impregnated with metal oxides and calcined at 300oC to form Zn/Al-TiO2 and Zn/Al-ZnO as photodegradation catalysts of congo red (CR). The characterization of the catalysts after preparation using SEM and UV-DRS while the catalyst that have been used in 5 regeneration cycles was characterized by XRD and FTIR. Photodegradation of CR was carried out by optimizing pH, catalyst weight, and time radiation. Zn/Al LDH which was modified into Zn/Al-TiO2 and ZnAl-ZnO had a better degradation percentage, rate constant, and stability than Zn/Al LDH pristine structure. Zn/Al LDH, Zn/Al TiO2 and Zn/Al-ZnO catalyzed CR photodegradation for 120 minutes with percent degradation 68.39%, 81.24% and 71.09%, respectively.
References
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Prince, J., F. Tzompantzi, G. Mendoza-Damián, F. Hernández-Beltrán, and J. S. Valente (2015). Photocatalytic Degradation of Phenol by Semiconducting Mixed Oxides Derived from Zn (Ga) Al Layered Double Hydroxides. Applied Catalysis B: Environmental, 163; 352–360
Qi, M., L. Fan, Y. Shen, H. Zou, X. Tian, D. Liu, and S. Li (2018). Improved Visible-Light-Induced Photocatalytic Performance of ZnAl Layered Double Hydroxide by Incorporation of Ni2+. Journal of Nanoscience and Nanotechnology, 18(1); 753–760
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Seftel, E., M. Niarchos, C. Mitropoulos, M. Mertens, E. Vansant, and P. Cool (2015). Photocatalytic Removal of Phenol and Methylene-Blue in Aqueous Media using TiO2@ LDH Clay Nanocomposites. Catalysis Today, 252; 120–127
Siregar, P. M. S. B. N., A. Lesbani, and R. Mohadi (2022). Mg/Al-Chitosan as a Selective Adsorbent in the Removal of Methylene Blue from Aqueous Solutions. Science and Technology Indonesia, 7(2); 170–178
Song, B., Z. Zeng, G. Zeng, J. Gong, R. Xiao, S. Ye, M. Chen, C. Lai, P. Xu, and X. Tang (2019). Powerful Combination of g-C3N4 and LDHs for Enhanced Photocatalytic Performance: a Review of Strategy, Synthesis, and Applications. Advances in Colloid and Interface Science, 272; 101999
Suárez-Quezada, M., G. Romero-Ortiz, V. Suárez, G. Morales-Mendoza, L. Lartundo-Rojas, E. Navarro-Cerón, F. Tzompantzi, S. Robles, R. Gómez, and A. Mantilla (2016). Photodegradation of Phenol using Reconstructed Ce Doped Zn/Al Layered Double Hydroxides as Photocatalysts. Catalysis Today, 271; 213–219
Trujillano, R., C. Nájera, and V. Rives (2020). Activity in the Photodegradation of 4-Nitrophenol of a Zn, Al Hydrotalcite-Like Solid and the Derived Alumina-Supported ZnO. Catalysts, 10(6); 702
Tzompantzi, F., G. Mendoza-Damián, J. Rico, and A. Mantilla (2014). Enhanced Photoactivity for the Phenol Mineralization on ZnAlLa Mixed Oxides Prepared from Calcined LDHs. Catalysis Today, 220; 56–60
Wang, X., P. Wu, Z. Huang, N. Zhu, J. Wu, P. Li, and Z. Dang (2014a). Solar Photocatalytic Degradation of Methylene Blue by Mixed Metal Oxide Catalysts Derived from ZnAlTi Layered Double Hydroxides. Applied Clay Science, 95; 95-103
Wang, X., P. Wu, Y. Lu, Z. Huang, N. Zhu, C. Lin, and Z. Dang (2014b). NiZnAl Layered Double Hydroxides as Photocatalyst Under Solar Radiation for Photocatalytic Degradation of Orange G. Separation and Purication Technology, 132; 195–205
Yan, R. D., G. H. Liu, Q. F. Wang, W. Liu, and C. L. Song (2016). Fast Photodegradation of Malachite Green using Nano-ZnO on Ceramic MgAl Carbonate Layered Double Hydroxides Support. Chinese Journal of Chemical Physics, 29(2); 241
Yuliasari, N., A. Wijaya, A. Amri, R. Mohadi, E. Elfita, and A. Lesbani (2022a). Application of M2+ (Magnesium, Zinc)/Alumina-Metal Oxide Composites as Photocatalysts for the Degradation of Cationic Dyes. Ecological Engineering & Environmental Technology; 4
Yuliasari, N., A. Wijaya, R. Mohadi, E. Elfita, and A. Lesbani (2022b). Photocatalytic Degradation of Malachite Green by Layered Double Hydroxide Based Composites. Bulletin of Chemical Reaction Engineering & Catalysis, 17(2); 240–249
Zhang, L., Z. Xiong, L. Li, R. Burt, and X. Zhao (2016). Uptake and Degradation of Orange II by Zinc Aluminum Layered Double Oxides. Journal of Colloid and Interface Science, 469; 224–230
Zhao, G., J. Zou, C. Li, J. Yu, X. Jiang, Y. Zheng, W. Hu, and F. Jiao (2018). Enhanced Photocatalytic Degradation of Rhodamine B, Methylene Blue and 4-Nitrophenol Under Visible Light Irradiation using TiO2/MgZnAl Layered Double Hydroxide. Journal of Materials Science: Materials in Electronics, 29(8); 7002–7014
Zhu, J., Z. Zhu, H. Zhang, H. Lu, Y. Qiu, L. Zhu, and S. Küppers (2016). Enhanced Photocatalytic Activity of Ce-Doped Zn-Al Multi-Metal Oxide Composites Derived from Layered Double Hydroxide Precursors. Journal of Colloid and Interface Science, 481; 144–157
Amor, F., A. Diouri, I. Ellouzi, F. Ouanji, and M. Kacimi (2018). High Efficient Photocatalytic Activity of Zn-Al-Ti Layered Double Hydroxides Nanocomposite. MATEC Web of Conferences, 149; 01087
Aoudjit, F., O. Cherifi, and D. Halliche (2019). Simultaneously Efficient Adsorption and Photocatalytic Degradation of Sodium Dodecyl Sulfate Surfactant by One-Pot Synthesized TiO2/Layered Double Hydroxide Materials. Separation Science and Technology, 54(7); 1095–1105
Bhuvaneswari, K., G. Palanisamy, T. Pazhanivel, T. Maiyalagan, and G. Bharathi (2019). Photodegradation Activity of Nitrogen-Rich Graphitic Carbon Nitride Intercalated ZnO/Mg-Al Layered Double Hydroxide Ternary Nanocomposites on Methylene Blue Dye. ChemistrySelect, 4(11); 2982–2990
Contreras-Ruiz, J., S. Martínez-Gallegos, J. García-Rivas, J. Illescas, J. González-Juárez, G. Macedo Miranda, and E. Ordonez Regil (2019). Influence of the Textural Parameters of LDH-TiO2 Composites on Phenol Adsorption and Photodegradation Capacities. International Journal of Photoenergy, 2019; 1–11
Djeda, R., G. Mailhot, and V. Prevot (2020). Porous Layered Double Hydroxide/TiO2 Photocatalysts for the Photocatalytic Degradation of Orange II. ChemEngineering, 4(2); 39
Elhalil, A., M. Sadiq, M. Abdennouri, Y. Kadmi, L. Favier, and N. Barka (2018). Synthesis of Ba Doped ZnO/Al2O3 Nanocomposite from Layered Double Hydroxide Structure and Their Photocatalytic Activity for the Degradation of Caffeine. Journal of Applied Surfaces and Interfaces, 4(1-3)
Gandamalla, A., S. Manchala, A. Verma, Y. P. Fu, and V. Shanker (2021). Microwave-Assisted Synthesis of ZnAl-LDH/g-C3N4 Composite for Degradation of Antibiotic Ciprofloxacin Under Visible-Light Illumination. Chemosphere, 283; 131182
Guzmán-Vargas, A., E. Lima, G. A. Uriostegui-Ortega, M. A. Oliver-Tolentino, and E. E. Rodríguez (2016). Adsorption and Subsequent Partial Photodegradation of Methyl Violet 2B on Cu/Al Layered Double Hydroxides. Applied Surface Science, 363; 372–380
Hadnadjev-Kostic, M., T. Vulic, R. Marinkovic-Neducin, D. Lončarević, J. Dostanić, S. Markov, and D. Jovanović (2017). Photo-Induced Properties of Photocatalysts: a Study on the Modified Structural, Optical and Textural Properties of TiO2-ZnAl Layered Double Hydroxide Based Materials. Journal of Cleaner Production, 164; 1–18
Huo, R., Y. Kuang, Z. Zhao, F. Zhang, and S. Xu (2013). Enhanced Photocatalytic Performances of Hierarchical ZnO/ZnAl2O4 Microsphere Derived from Layered Double Hydroxide Precursor Spray-Dried Microsphere. Journal of Colloid and Interface Science, 407; 17–21
Kim, S., J. Fahel, P. Durand, E. André, and C. Carteret (2017). Ternary Layered Double Hydroxides (LDHs) Based on Co-, Cu-Substituted ZnAl for the Design of Efficient Photocatalysts. European Journal of Inorganic Chemistry, 2017(3); 669–678
Li, D., L. Fan, M. Qi, Y. Shen, D. Liu, and S. Li (2018). Enhanced Visible-Light-Driven Photocatalytic Activity of ZnAl Layered Double Hydroxide by Incorporation of Co2+. Bulletin of Chemical Reaction Engineering & Catalysis, 13(3); 502
Li, Z., M. Chen, H. Hu, Q. Zhang, and D. Tao (2020). Mechanochemical Synthesis of Novel Pt Modified ZnAl-LDH for Effective Ciprofloxacin Photodegradation. Journal of Solid State Chemistry, 290; 121594
Morales-Mendoza, G., F. Tzompantzi, C. Garcia Mendoza, R. Lopez, V. De la Luz, S. W. Lee, T. H. Kim, L. M. Torres-Martinez, and R. Gomez (2015). Mn-Doped Zn/Al Layered Double Hydroxides as Photocatalysts for the 4-Chlorophenol Photodegradation. Applied Clay Science, 118; 38–47
Mourid, E. H., L. El Mersly, L. Benaziz, S. Rafqah, M. Lakraimi, et al. (2020). Development of a New Recyclable Nanocomoposite LDH-TiO2 for the Degradation of Antibiotic Sulfamethoxazole Under UVA Radiation: an Approach Towards Sunlight. Journal of Photochemistry and Photobiology A: Chemistry, 396; 112530
Muhammad, A. and F. Garzali (2019). Photodegradation of Rhodamine B using Cd-Al/C Double Layered Hydroxide Catalyst. Bayero Journal of Pure and Applied Sciences, 12(1); 24–30
Nandiyanto, A. B. D., R. Oktiani, and R. Ragadhita (2019). How to Read and Interpret FTIR Spectroscope of Organic Material. Indonesian Journal of Science and Technology, 4(1); 97–118
Prince, J., F. Tzompantzi, G. Mendoza-Damián, F. Hernández-Beltrán, and J. S. Valente (2015). Photocatalytic Degradation of Phenol by Semiconducting Mixed Oxides Derived from Zn (Ga) Al Layered Double Hydroxides. Applied Catalysis B: Environmental, 163; 352–360
Qi, M., L. Fan, Y. Shen, H. Zou, X. Tian, D. Liu, and S. Li (2018). Improved Visible-Light-Induced Photocatalytic Performance of ZnAl Layered Double Hydroxide by Incorporation of Ni2+. Journal of Nanoscience and Nanotechnology, 18(1); 753–760
Rudic, O., J. Ranogajec, T. Vulic, S. Vucetic, D. Cjepa, and D. Lazar (2014). Photo-Induced Properties of TiO2/ZnAl Layered Double Hydroxide Coating Onto Porous Mineral Substrates. Ceramics International, 40(7); 9445–9455
Seftel, E., M. Niarchos, C. Mitropoulos, M. Mertens, E. Vansant, and P. Cool (2015). Photocatalytic Removal of Phenol and Methylene-Blue in Aqueous Media using TiO2@ LDH Clay Nanocomposites. Catalysis Today, 252; 120–127
Siregar, P. M. S. B. N., A. Lesbani, and R. Mohadi (2022). Mg/Al-Chitosan as a Selective Adsorbent in the Removal of Methylene Blue from Aqueous Solutions. Science and Technology Indonesia, 7(2); 170–178
Song, B., Z. Zeng, G. Zeng, J. Gong, R. Xiao, S. Ye, M. Chen, C. Lai, P. Xu, and X. Tang (2019). Powerful Combination of g-C3N4 and LDHs for Enhanced Photocatalytic Performance: a Review of Strategy, Synthesis, and Applications. Advances in Colloid and Interface Science, 272; 101999
Suárez-Quezada, M., G. Romero-Ortiz, V. Suárez, G. Morales-Mendoza, L. Lartundo-Rojas, E. Navarro-Cerón, F. Tzompantzi, S. Robles, R. Gómez, and A. Mantilla (2016). Photodegradation of Phenol using Reconstructed Ce Doped Zn/Al Layered Double Hydroxides as Photocatalysts. Catalysis Today, 271; 213–219
Trujillano, R., C. Nájera, and V. Rives (2020). Activity in the Photodegradation of 4-Nitrophenol of a Zn, Al Hydrotalcite-Like Solid and the Derived Alumina-Supported ZnO. Catalysts, 10(6); 702
Tzompantzi, F., G. Mendoza-Damián, J. Rico, and A. Mantilla (2014). Enhanced Photoactivity for the Phenol Mineralization on ZnAlLa Mixed Oxides Prepared from Calcined LDHs. Catalysis Today, 220; 56–60
Wang, X., P. Wu, Z. Huang, N. Zhu, J. Wu, P. Li, and Z. Dang (2014a). Solar Photocatalytic Degradation of Methylene Blue by Mixed Metal Oxide Catalysts Derived from ZnAlTi Layered Double Hydroxides. Applied Clay Science, 95; 95-103
Wang, X., P. Wu, Y. Lu, Z. Huang, N. Zhu, C. Lin, and Z. Dang (2014b). NiZnAl Layered Double Hydroxides as Photocatalyst Under Solar Radiation for Photocatalytic Degradation of Orange G. Separation and Purication Technology, 132; 195–205
Yan, R. D., G. H. Liu, Q. F. Wang, W. Liu, and C. L. Song (2016). Fast Photodegradation of Malachite Green using Nano-ZnO on Ceramic MgAl Carbonate Layered Double Hydroxides Support. Chinese Journal of Chemical Physics, 29(2); 241
Yuliasari, N., A. Wijaya, A. Amri, R. Mohadi, E. Elfita, and A. Lesbani (2022a). Application of M2+ (Magnesium, Zinc)/Alumina-Metal Oxide Composites as Photocatalysts for the Degradation of Cationic Dyes. Ecological Engineering & Environmental Technology; 4
Yuliasari, N., A. Wijaya, R. Mohadi, E. Elfita, and A. Lesbani (2022b). Photocatalytic Degradation of Malachite Green by Layered Double Hydroxide Based Composites. Bulletin of Chemical Reaction Engineering & Catalysis, 17(2); 240–249
Zhang, L., Z. Xiong, L. Li, R. Burt, and X. Zhao (2016). Uptake and Degradation of Orange II by Zinc Aluminum Layered Double Oxides. Journal of Colloid and Interface Science, 469; 224–230
Zhao, G., J. Zou, C. Li, J. Yu, X. Jiang, Y. Zheng, W. Hu, and F. Jiao (2018). Enhanced Photocatalytic Degradation of Rhodamine B, Methylene Blue and 4-Nitrophenol Under Visible Light Irradiation using TiO2/MgZnAl Layered Double Hydroxide. Journal of Materials Science: Materials in Electronics, 29(8); 7002–7014
Zhu, J., Z. Zhu, H. Zhang, H. Lu, Y. Qiu, L. Zhu, and S. Küppers (2016). Enhanced Photocatalytic Activity of Ce-Doped Zn-Al Multi-Metal Oxide Composites Derived from Layered Double Hydroxide Precursors. Journal of Colloid and Interface Science, 481; 144–157
Authors
Yuliasari, N., Amri, Mohadi, R., Elfita, E., & Lesbani, A. (2022). Improvement of Congo Red Photodegradation Performance Through Zn/Al-TiO2 and Zn/Al-ZnO Preparation. Science and Technology Indonesia, 7(4), 449–454. https://doi.org/10.26554/sti.2022.7.4.449-454
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